Low Dimensional Quantum Structure Lasers

 

Staffs:      Y. Suematsu S. Arai         S. Tamura

Post-Doctoral Research Fellow:                        B. Chen           N. Nunoya (from Oct.)

Students:     N. Nunoya                     M. Morshed    H. Yagi             K. Muranushi   K. Ohira                                   A. Onomura     T. Sano

 

GaInAsP/InP strained-quantum-film, -wire and -box lasers have been studied. Distributed feedback (DFB) lasers consisting of wirelike active regions fabricated by the same fabrication process as Quantum-Wire lasers have been also studied.

Results obtained in this research are as follows:

 

(1)      1.5-mm-wavelength partially strain-compensated GaInAsP/InP 5-layered quantum-wire lasers with the wire width of 23 nm in the period of 80 nm were realized for the first time by electron beam lithography, CH4/H2-reactive ion etching and organometallic vapor-phase-epitaxial regrowth. The threshold current density of 774 A/cm2 and differential quantum efficiency of 40 % were obtained under a pulsed condition at room temperature. From measurement of spontaneous emission spectra, the blue shift at the peak wavelength was 38 meV, which was much larger than a calculated value, and the spontaneous emission spectral width was almost constant at temperatures between 103 K and 253 K, indicating a lateral quantum confinement effect. Finally, the spontaneous emission efficiency below the threshold was almost comparable to that of the Q-Film lasers up to 85 °C, that revealed low-damage property of the etched/regrown interfaces.

(2)      GaInAsP/InP partially strain-compensated multiple-quantum-wire lasers with the wire widths of 18 nm and 27 nm in the period of 80 nm were also realized. Size fluctuations of these quantum-wire structures were measured by scanning electron microscope views, from which the standard deviation was obtained to be less than 2 nm. The differential quantum efficiencies of these quantum-wire lasers were almost the same as that of the 5-quantum-well lasers at room temperature. From EL spectra of various wire widths lasers, a larger energy blue shift than that from a simple analysis model was observed, which can be attributed to residual compressive strain between the active region and surrounding InP layer.

(3)      High-performance operation of 1.55 mm wavelength GaInAsP/InP strongly index-coupled and gain-matched distributed feedback lasers with periodic wirelike active regions was realized, whose index-coupling coefficient was more than 300 cm-1. In order to design lasers for low threshold current operation, threshold current dependences on the number of quantum wells and the wire width were investigated both theoretically and experimentally. A record low threshold current of 0.7 mA was realized at room temperature CW condition for a 2.3-mm-wide buried heterostructure with a 200-mm-long cavity. We also confirmed stable single-mode operation due to a gain matching effect between the standing-wave profile and the wirelike active region.

(4)      A CW life test of 1550 nm gain-matched DFB laser, which consists of wire-like active regions and exhibits sub-mA threshold, was carried out. No degradation was observed in the output and the spectral characteristics after 8500 hrs operation at a bias current around 10 times the threshold.

(5)      A distributed reflector (DR) laser consisting of wirelike active regions with asymmetric output characteristic was realized for the first time. To realize an asymmetric output property while maintaining low threshold current operation, a l/4 shifted grating and modulated active region widths were introduced into the grating structure. Threshold current as low as 1.8 mA, asymmetric output ratio of 8, and a sub-mode suppression-ratio (SMSR) of 33 dB at I=1.2Ith were obtained for the cavity length of 200 mm and the stripe width of 2.3 mm under a RT-CW condition.

 


New Types of Semiconductor Lasers for Photonic Integration

 

Staffs:    Y. Suematsu              S. Arai       S. Tamura

Post-Doctoral Research Fellow:                        B. Chen           N. Nunoya (from Oct.)

Students:     J. Wiedmann   N. Nunoya                    H.-C. Kim       K. Ebihara       K. Matsui                                                     T. Okamoto                    M. Ohta          Y. Onodera      H. Kanjo

 

Semiconductor lasers with low threshold current, high efficiency, and single wavelength operation are very attractive for optical interconnection and a number of optoelectronics applications. New types of semiconductor lasers, such as multiple-micro-cavity (MMC) lasers, deeply etched distributed-Bragg-reflector (DBR) and vertical-grating distributed feedback (VG-DFB) lasers as well as vertical-grating distributed-reflector (VG-DR) lasers have been studied both theoretically and experimentally.

Membrane lasers consisting of very thin semiconductor core layer sandwiched by polymer/SiO2 cladding layers have been also studied.

Results obtained in this research are as follows:

 

(1)      High-reflectivity semiconductor/BCB reflectors were fabricated by multiple sequential steps of CH4/H2 RIE etching and O2 plasma ashing. The reflectivity was estimated to be as high as 95%. Using these reflectors, highly uniform 1.55-mm-wavelength lasers with low threshold and high differential quantum efficiency were demonstrated. In addition, the reliability of such polymer-buried DBR lasers was investigated for the first time. The technology employed in this work is highly promising for the monolithic integration and batch processing of edge emitting lasers with other photonic devices through low-loss polymer waveguides.

(2)      The novel design for obtaining single-mode operation by combing a DBR facet with multiple cavities was analyzed in theory and experiment. It was shown that the loss per groove is an important parameter for the best choice of the cavity number. Single-mode operation was obtained for different number of cavities. Increasing the number of cavities will decrease the efficiency drastically. The threshold current is lowest for two or three cavities. Therefore, it can be concluded that a CC laser is best for laser operation according to high efficiency and low threshold. For the CC laser an SMSR of 36dB was achieved at 1.8 Ith.

(3)      A novel DR laser including a vertically etched grating was successfully fabricated. In case of a mesa width of WS = 6 mm and mesa width variation of DWS = 0.5 mm,  a low threshold current of Ith = 12.4 mA and a high differential quantum efficiency of hd = 42% were achieved with an SMSR of 33 dB.

(4)      Distributed feedback lasers with a deeply etched first order vertical grating were realized for the first time. It was shown that we could obtain an effective coupling by reducing the stripe width. The sample with the cavity length of 430 mm, 1.8 mm stripe width and 0.2 mm grating depth on each lateral side exhibited a 12.5 mA threshold current, 37 % total differential quantum efficiency and an SMSR of 35 dB at a bias current of two times the threshold.

(5)      By use of VG-DFB structure, it was clarified that structural birefringence can be completely eliminated. The grating coupling coefficient can also be polarization independent by adjusting grating depth.

(6)      Novel semiconductor laser structure, that is, membrane laser which has the Benzocyclobutene (BCB) cladding layers, enables to increase optical confinement into active layer due to a large refractive index difference between the active and cladding layers. A RT-CW operation of membrane DFB laser consisting of deeply etched single-quantum-well wirelike active regions was demonstrated for the first time under optical pumping. A threshold power of 38 mW was obtained for 10.7 mm-wide and 40 mm-long device. From spontaneous emission spectrum, a large stop-band width of 65 nm and a low equivalent refractive index of 2.30, which are peculiar to a thin membrane waveguide structure, were observed.

(7)      In order to realize single mode and low threshold operation of 1.5 mm-wavelength GaInAsP/InP membrane DFB laser, buried heterostructure (BH) was innovated by slightly changing the fabrication process. A threshold pump power of 4.8 mW and an SMSR of 39 dB were obtained for a 142 nm-thick semiconductor membrane core layer with a cavity length of 120 mm and a stripe width of 2 mm under RT-CW optical pumping. The corresponding threshold for current injection was roughly estimated to be 88 mA.

 


Quantum Coherent Electron Devices

 

Staffs:                      K. Furuya  Y.Miyamoto  N.Machida  S. Tamura

Visiting Researcher:          B. Zhang

Post-Doctoral Research Fellow:                        M. Nagase (from Oct.)

Students:  M. Nagase  S. Karasawa  M. Kurahashi H. Oguchi

                     T. Hirata  R. Yamamoto  H. Nakamura T. Okada 

                     K. Mae  H. Maeda    H. Nagatsuka  Y. Ninomiya

                     M. Fukasawa  D. Miyamoto  K. Takeuchi

 

Ballistic transport of hot electron has a possibility of new high-speed and functional devices using wave property of electron. We studied wave properties of hot electron for new principle of electron devices.

Results obtained in this research are as follows:

 

(1) The solid-state biprism is a solid-state version of the vacuum biprism that has been realized, and is also proposed as a test ground for electron interference observation and a new conceptual device. Toward the device, consecutive numerical simulation essential to discuss observation of hot electron interference in solid-state biprism has been performed. Two dimensional quantum beam propagation method was used to calculate electron wavefunction when there exists magnetic field. As results, it was found that magnetic field in a range from 0 to 0.3 T shifted interference pattern of hot electron in space and application of magnetic field in this range enables us to detect hot electron interference when transverse energy spread of incident electron flux is 0.3 meV.

(2) To eject electron wave with high lateral coherence into an active device region, a coherent emitter has been proposed. By introducing an additional electrode, the gate, to a double-barrier resonant-tunneling emitter, an electron flux with a single wavelength, a wide wavefront spread, and high current density can be achieved. This emitter can also be used for various types of solid-state spectroscopy.

(3) We have proposed a novel transistor where hot electrons are generated and travel through undoped semiconductor region by adopting a combination of double-barrier resonant-tunneling structure and metal wire, and we have attempted to demonstrate attractive potential formation required in operation of the biprism by our proposed transistor. After fundamental studies of crystal growth for resonant-tunneling structure and burying metal in semiconductors, we have fabricated the device by re-growth to bury Tungsten in GaAs using OMVPE. By analysis of measured data, for the first time, a formation of attractive potential around the buried metal wire has been demonstrated. Furthermore, to reduce emitter-gate leakage current, we have fabricated transistors on InP semi-insulating substrate and wired by free-standing wire. From measured I-V characteristics, it has been shown that buried metal wire gate has enabled to produce attractive potential and leakage current has been reduced by examining value of peak current at negative differential resistance. Therefore, we have been able to show the potential of our device.

(4) Based on reciprocity theorem of quantum mechanics, a new experimental method using ballistic electron emission microscopy (BEEM) for observation of electron wave diffraction in semiconductor has been proposed and numerical simulations of the experiment have been performed in order to clarify conditions for the observation. A material combination of GaInAs/InP showed a clear diffraction pattern due to a phase shift structure as a cause of wavefront modulation. The diffraction pattern still appeared when energy spread of 200 meV of electrons in BEEM current was assumed. This energy spread allows BEEM current to be over 1 pA when tunneling current is set to 10 nA and the current level is large enough to be detected by ordinal BEEM system.

(5) To explore a possibility of phase coherence estimations of hot electron in semiconductors, current-voltage (I-V) characteristics of triple-barrier resonant-tunneling diodes (TBRTDs) have been studied. The current peak broadening caused by the well-well coupling and well-electrode coupling was revealed. The electron phase breaking effect was incorporated into the analysis to obtain the I-V curve of TBRTD using the phase correlation method. For strong well-well coupling, the peak current was independent of the phase breaking, while for weak coupling it is dependent on it. Therefore, the electron coherence can be estimated using TBRTD designed appropriately.

 


High-Speed Electron Devices Using Advanced Structures and Materials

 

Staffs:    K. Furuya   M. Asada    Y. Miyamoto   M. Watanabe   S. Tamura

Students:        T.Arai  M.Tsutsui  K. Hoshina  M. Saitoh  N. Sashinakai

               S. Yamagami  T. Abe  T. Morita  H. Sato  R. Yamamoto

                     Y. Fujioka  K. Kashima  Y. Kontani  K. Matsuda  T. Nagai

                     H. Nagatsuka  N. Orihashi  T. Sakai  H. Sato  K. Yokoyama

 

Superlattices and ultrathin layers with the combination of metal and insulator were proposed as one of the candidates of the material for ultrahigh-speed electronic devices and optical devices because of the low resistivity of metals, low dielectric constant and wide band gap of insulators and high conduction band offset at metal/insulator heterointerface. A novel transistor using quantum interference in metal/insulator heterostructure has been proposed and it was shown theoretically that sub-pico second response could be expected in such devices.

Results obtained up to now are as follows:

 

(1)    The Schottky source/drain (S/D) MOSFET has the potential for scaling into the nanometer regime, because low electrode resistances with very shallow extension can be realized using metal source/drain. Very short channel Schottky S/D MOSFET with SOI structure were analyzed theoretically. The short channel effect can be suppressed even with a 15 nm-long channel at tOX = 1 nm and tSOI = 3 nm. The very short channel devices with metal gate (ErSi2 for n-type, and PtSi for p-type) were fabricated on SIMOX substrate, and the room temperature operation of sub 50nm devices was demonstrated. For 25 nm-long gate p-type devices, comparable drivability to conventional MOSFETs was archived with the drain current of -293 mA/mm and the transconductance of 431mS/mm at VDS = VGS = -1.5 V. The on/off ration was improved by using a very thin 35nm-thick SOI structure.

(2)    Current change under irradiation of a terahertz electromagnetic wave was measured for a triple-barrier resonant tunneling diodes integrated with a planar patch antenna. Gradual change from the classical square-law detection to photon-assisted tunneling with increasing photon energy was observed. The intersubband THz gain due to electron transition between adjacent quantum wells was estimated using the measurement of current change. Estimated gain at room temperature was ~0.15cm-1 at 1.4THz for a sample with relatively thick separation layer.

(3)    A GaInAs/InP buried metal heterojunction bipolar transistors (BM-HBTs) with a 0.3-µm-wide emitter was fabricated by electron-beam lithography, in which tungsten stripe with the same area as the emitter was buried with an intrinsic collector layer. Total base collector capacitance was reduced to about 30% of that calculated from physical dimensions of a conventional HBTs. Minimum total base collector capacitance was less than 1fF..

(4)    Fabrication process for narrow emitter along <010> direction in heterojunction bipolar transistor fully drawn by electron beam lithography was studied. Emitter structure of a 100 nm width was formed by using a combination of dry etching and wet etching. .Current gain of 51 was observed in the HBT with 0.1-μm-wide emitter was confirmed. To our knowledge, this emitter width of HBT is the smallest.

 


Light Emitting Devices Using Advanced Structures and Materials

 

Staff:          M. Watanabe

Students:     T. Maruyama   S. Okano         N. Sakamaki                    M.Suzuki

                    T. Ishikawa      N. Nakamura   Y. Niiyama                    M. Matsusda

                    D. Okamoto     T. Kanazawa

 

New type of light emitting devices using quantum-nano structures are studied. Intersubband quantum cascade lasers using CdF2-CaF2 heterostructures have been proposed and formation of sharp energy subbands in the quantum wells has been confirmed using resonant tunneling diode structures. Novel candidate for lattice-matched, wide-bandgap compound semiconductor Be-chalcogenides was proposed and epitaxial growth of high-Be-content BeZnSe was demonstrated.

Results obtained in this research are as follows.

 

(1) In order to realize intersubband cascade lasers, it is essential to control energy levels of subbands in CdF2 or Si quantum wells confined by CaF2 energy barriers. This year, nanoarea local epitaxy (NLE) was proposed to grow CdF2-CaF2 double barrier resonant tunneling diode (RTD) structures. The fine hole arrays of 100 nm in diameter was formed on a 15 nm-thick SiO2 layer on Si substrate with 0.1° off miscutt angle using electron beam lithography. This yields atomically flat Si surface with no atomic steps in growth region, which is essential to grow pinhole-free 1 nm-thick CaF2 for tunneling barrier layers. In the result, uniformity of the I-V characteristics and stability of the device performance was dramatically enhanced. And moreover, energy subband control by changing CdF2-QW thickness was firstly demonstrated.

(2) Epitaxial growth and room temperature negative differential resistance (NDR) of CdF2-CaF2 double barrier resonant tunneling diode (RTD) on Si(100) substrate was successfully achieved for the first time. To control inhomogeneous migration of CaF2, hydrogen terminated Si(100) was prepared and CaF2 was gown at 300°C, which yields atomically flat CaF2 epilayers on Si(100) substrate. Based on the CaF2, DBRTD structure was fabricated and NDR with peak-to-valley current ratio (PVCR) = 4.3 was observed at room temperature for the first time.

(3) The epitaxial growth of zinc oxide (ZnO) nanocrystals embedded in a single-crystalline CaF2 layer on a Si(111) substrate has been demonstrated. Highly c-axis-oriented ZnO 4-10 nm thick was grown on a CaF2(111) layer using radio-frequency (RF) sputtering followed by annealing in ultrahigh vacuum, resulting in the formation of epitaxial self-organized ZnO nanocrystals on CaF2/Si(111). It was found that CaF2 can be grown epitaxially over ZnO/CaF2 by molecular beam epitaxy (MBE), thus the CaF2/ZnO/CaF2 heterostructure has been formed on a Si(111) substrate. Abrupt heterointerfaces between CaF2 and ZnO were confirmed on a transmission electron microscope (TEM) cross section, and ultraviolet (UV) photoluminescence (PL) corresponding to the band-gap energy of ZnO was dominant in PL spectra observed at room temperature.

(4) Be-chalcogenides II-VI semiconductors is good candidate for the materials of long life-time II-VI lasers because of the strong covalent bonding of Be. Moreover, BeMgZnSe quaternary compound semiconductor can be lattice matched to Si and its energy band gap covers UV region (290-345nm). This year, BexZn1-xSe (x=0.2-1.0) was grown on CaF2/Si(111) and GaP(001) substrate by MBE at growth temperature of 250oC. The crystalline quality and surface morphology of BeZnSe/GaP(001) were better than the one of BeZnSe/CaF2/Si(111). Single crystalline and atomically flat BeZnSe on GaP(001) was obtained at 250oC, 0.1 mm/h and VI/II=1. UV photoluminescence was observed from band edge at 17K and room temperature. The growth of BeMgZnSe on GaP(001) was also obtained. Crystalline quality of BeMgZnSe was maintained until Mg content of around 15 %. This result, which was contained in high Mg content, was obtained for the first time.

 


Processing for Nanometer Structures

 

Staffs:         K. Furuya   S. Arai   Y. Miyamoto   M. Watanabe   S. Tamura

Students:    T. Arai       H. Oguchi        S. Yamagami  T. Morita        H. Nakamura 

Y. Okuda   R. Yamamoto     H. Maeda        T. Ninomiya     K. Takeuchi                       K. Yokoyama

 

Study of nanometer structure fabrication technology is important for the realization of quantum effect devices such as quantum-wire, or –box devices and ballistic electron devices based on wave characteristics of electrons.

Results obtained in this research are as follows:

 

(1)          Contact characteristics and isolation characteristics of 80-nm-period fine electrodes were reported. By using Au/Ti as electrodes and 2×1019 cm-3 as a carrier concentration of n-GaInAs, observed contact resistivity was less than 1.5×10-4 Wcm2. By using etching of n-GaInAs layer and band discontinuity in undoped isolation characteristics satisfied the condition to observe an interference pattern of hot electron.